Ionic capillary evaporation in weakly charged nanopores.

Sahin Buyukdagli, Manoel Manghi, John Palmeri
Author Information
  1. Sahin Buyukdagli: Laboratoire de Physique Théorique-IRSAMC, CNRS and Université de Toulouse, UPS, F-31062 Toulouse, France.

Abstract

Using a variational field theory, we show that an electrolyte confined to a neutral cylindrical nanopore traversing a low dielectric membrane exhibits a first-order ionic liquid-vapor pseudo-phase-transition from an ionic-penetration "liquid" phase to an ionic-exclusion "vapor" phase, controlled by nanopore-modified ionic correlations and dielectric repulsion. For weakly charged nanopores, this pseudotransition survives and may shed light on the mechanism behind the rapid switching of nanopore conductivity observed in experiments.

MeSH Term

Electrolytes
Ions
Nanopores
Static Electricity
Volatilization

Chemicals

Electrolytes
Ions