Stable Low-Bandgap Pb-Sn Binary Perovskites for Tandem Solar Cells.

Zhibin Yang, Adharsh Rajagopal, Chu-Chen Chueh, Sae Byeok Jo, Bo Liu, Ting Zhao, Alex K-Y Jen
Author Information
  1. Zhibin Yang: Department of Materials Science and Engineering, University of Washington, Seattle, WA, 98195-2120, USA.
  2. Adharsh Rajagopal: Department of Materials Science and Engineering, University of Washington, Seattle, WA, 98195-2120, USA.
  3. Chu-Chen Chueh: Department of Materials Science and Engineering, University of Washington, Seattle, WA, 98195-2120, USA.
  4. Sae Byeok Jo: Department of Materials Science and Engineering, University of Washington, Seattle, WA, 98195-2120, USA.
  5. Bo Liu: Department of Materials Science and Engineering, University of Washington, Seattle, WA, 98195-2120, USA.
  6. Ting Zhao: Department of Materials Science and Engineering, University of Washington, Seattle, WA, 98195-2120, USA.
  7. Alex K-Y Jen: Department of Materials Science and Engineering, University of Washington, Seattle, WA, 98195-2120, USA. ajen@u.washington.edu.

Abstract

A low-bandgap (1.33 eV) Sn-based MA FA Pb Sn I perovskite is developed via combined compositional, process, and interfacial engineering. It can deliver a high power conversion efficiency (PCE) of 14.19%. Finally, a four-terminal all-perovskite tandem solar cell is demonstrated by combining this low-bandgap cell with a semitransparent MAPbI cell to achieve a high efficiency of 19.08%.

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