I and its species in the East China Sea: level, distribution, sources and tracing water masses exchange and movement.

Dan Liu, Xiaolin Hou, Jinzhou Du, Luyuan Zhang, Weijian Zhou
Author Information
  1. Dan Liu: State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Cademy of Sciences, Xi'an 710061, China.
  2. Xiaolin Hou: State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Cademy of Sciences, Xi'an 710061, China.
  3. Jinzhou Du: State Key Laboratory of Estuarine and Coastal Research, East China Normal University, Shanghai, 200062, China.
  4. Luyuan Zhang: State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Cademy of Sciences, Xi'an 710061, China.
  5. Weijian Zhou: State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Cademy of Sciences, Xi'an 710061, China.

Abstract

Anthropogenic I as a long-lived radioisotope of iodine has been considered as an ideal oceanographic tracer due to its high residence time and conservative property in the ocean. Surface water samples collected from the East China Sea (ECS) in August 2013 were analyzed for I, I and their inorganic chemical species in the first time. The measured I/I ratio is 1-3 orders of magnitude higher than the pre-nuclear level, indicating its dominantly anthropogenic sources. Relatively high I levels were observed in the Yangtze River and its estuary, as well as in the southern Yellow Sea, and I level in seawater declines towards the ECS shelf. In the open sea, I and I in surface water exists mainly as iodate, while in Yangtze River estuary and some locations, iodide is dominated. The results indicate that the Fukushima nuclear accident has no detectable effects in the ECS until August 2013. The obtained results are used for investigation of interaction of various water masses and water circulation in the ECS, as well as the marine environment in this region. Meanwhile this work provides essential data for evaluation of the possible influence of the increasing NPPs along the coast of the ECS in the future.

References

  1. Environ Sci Technol. 2013 Sep 3;47(17):9693-8 [PMID: 23931086]
  2. Anal Chim Acta. 2009 Jan 26;632(2):181-96 [PMID: 19110092]
  3. Microbes Environ. 2008;23(4):269-76 [PMID: 21558718]
  4. Mar Pollut Bull. 2001 Dec;42(12):1347-56 [PMID: 11827122]
  5. J Environ Radioact. 2013 Dec;126:45-54 [PMID: 23954281]
  6. Sci Total Environ. 2010 Oct 1;408(21):5052-64 [PMID: 20692686]
  7. J Environ Radioact. 2016 Apr;154:15-24 [PMID: 26821329]
  8. Anal Chem. 2013 Apr 2;85(7):3715-22 [PMID: 23472747]
  9. Environ Sci Technol. 2014;48(3):1419-25 [PMID: 24359222]
  10. Environ Sci Technol. 2011 Feb 1;45(3):903-9 [PMID: 21190361]
  11. Sci Rep. 2013 Nov 28;3:2685 [PMID: 24284916]
  12. Environ Sci Process Impacts. 2015 May;17(5):932-8 [PMID: 25901961]
  13. Sci Total Environ. 2000 Feb 10;246(2-3):285-91 [PMID: 10696729]
  14. Environ Sci Technol. 2015 Jun 2;49(11):6691-700 [PMID: 25944707]
  15. Environ Sci Technol. 2007 Sep 1;41(17):5993-9 [PMID: 17937272]
  16. Environ Sci Technol. 2013 Aug 6;47(15):8383-90 [PMID: 23829385]
  17. Huan Jing Ke Xue. 2015 Jun;36(6):2019-27 [PMID: 26387303]
  18. Anal Chem. 2010 Sep 15;82(18):7713-21 [PMID: 20735008]
  19. Environ Sci Technol. 2013 Apr 2;47(7):3091-8 [PMID: 23461388]
  20. Environ Sci Technol. 2014 Mar 18;48(6):3136-44 [PMID: 24564849]

Word Cloud

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