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Angewandte Chemie (International ed. in English)
May 10, 2021;60 (20): 11048-11067.

Metal-Organic Framework Derived Bimetallic Materials for Electrochemical Energy Storage.

Soheila Sanati, Reza Abazari, Josep Albero, Ali Morsali, Hermenegildo García, Zibin Liang, Ruqiang Zou
Author Information
  1. Soheila Sanati: Department of Chemistry, Faculty of Basic Sciences, Tarbiat Modares University, Tehran, 14115-175, Iran.
  2. Reza Abazari: Department of Chemistry, Faculty of Basic Sciences, Tarbiat Modares University, Tehran, 14115-175, Iran.
  3. Josep Albero: Dep. Instituto Universitario de Tecnología Química (CSIC-UPV), Universitat Politècnica de València, València, 46022, Spain. ORCID
  4. Ali Morsali: Department of Chemistry, Faculty of Basic Sciences, Tarbiat Modares University, Tehran, 14115-175, Iran.
  5. Hermenegildo García: Dep. Instituto Universitario de Tecnología Química (CSIC-UPV), Universitat Politècnica de València, València, 46022, Spain. ORCID
  6. Zibin Liang: Beijing Key Lab of Theory and Technology for Advanced Battery Materials, Department of Materials Science and Engineering, College of Engineering, Peking University, Beijing, 100871, China.
  7. Ruqiang Zou: Beijing Key Lab of Theory and Technology for Advanced Battery Materials, Department of Materials Science and Engineering, College of Engineering, Peking University, Beijing, 100871, China.
PMID: 32910529 DOI: 10.1002/anie.202010093

Abstract

Supercapacitors (SCs), showing excellent power density, long service life, and high reversibility, have received great attention because of the increasing demand for energy storage devices. To further improve their performance, it is essential to develop advanced electrode materials. One group of materials, porous crystalline solids referred to as metal-organic frameworks (MOFs), have proved to be excellent templates for synthesizing functional materials to be employed in the preparation of electrodes for SCs. In comparison to monometallic MOFs, bimetallic MOFs and their derivatives offer a number of advantages, including tunable electrochemical activity, high charge capacity, and improved electrical conductivity. This review focuses on the use of MOF-derived bimetallic materials in SCs, the origin of the improved performance, and the latest developments in the field. Furthermore, the challenges and perspectives in this research area are discussed.

Keywords

bimetallic materials electrode materials energy storage metal-organic frameworks supercapacitors

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Grants

  1. Severo Ochoa/Ministerio de Ciencia e Innovación
  2. RTI2018-89237/Ministerio de Ciencia e Innovación
  3. Prometeo 2017-083/Generalitat Valenciana
  4. /Tarbiat Modares University
  5. /Peking University
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