Synthesis and in vitro activity of novel quaternary ammonium carbapenems: 2-pyridiniopropyl and 1-pyridinioethyl carbapenems.

Y Ueda, V Vinet
Author Information
  1. Y Ueda: Antiinfective Chemistry Department, Bristol-Myers Squibb Company, Candiac, Quebec, Canada.

Abstract

The synthesis of new carbapenems having either a pyridiniopropyl group at the 2-position or a pyridinioethyl group at the 1-position is described, along with the preparation of their corresponding hydroxy and acetoxy analogs. The antibacterial activity, susceptibility to dehydropeptidase-I (DHP-I) enzyme and chemical stability of these new carbapenems are also reported. 2-Pyridiniopropyl-carbapenem 4 was found to possess excellent antibacterial activity. It was more stable chemically and less susceptible to the DHP-I enzyme than the thio analog 3. 1-Pyridinioethylcarbapenem 5 showed significantly reduced antibacterial activity as compared to 2-pyridiniopropylcarbapenem 4.

MeSH Term

Carbapenems
Drug Stability
Molecular Conformation
Structure-Activity Relationship

Chemicals

Carbapenems

Word Cloud

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